Effect of nitrogen compounds on transport of ruthenium through the RCS

نویسندگان

  • Ivan Kajan
  • Teemu Kärkelä
  • Ari Auvinen
  • Christian Ekberg
چکیده

Ruthenium is a fission product that can be released from the fuel in case of a severe nuclear accident. In this work the impact of the atmosphere composition, including air radiolysis products, on the transport of ruthenium through a primary circuit was examined. Experiments were performed at temperatures 1300, 1500 and 1700 K in a slightly humid air. In the experiments significant effect of nitrogen oxides (N2O, NO2) and nitric acid on the ruthenium chemistry in the model primary circuit was observed. The obtained results indicate a strong effect of air radiolysis products on the quantity partitioning of transported ruthenium to gaseous and aerosol compounds.

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عنوان ژورنال:

دوره 311  شماره 

صفحات  -

تاریخ انتشار 2017